Issues and priorities
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Consistent operation of existing observing systems is necessary to detect the eventual recovery of the ozone layer, not expected before 2020.
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New satellite instruments were started recently and will give a substantial increase in data coverage. However, long-term validation and consistency of these instruments needs to be ascertained.
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There is a need for improved distribution and calibration of ground-based observations to support the use of satellite data for global monitoring of ozone.
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Existing multiple data centres should be better integrated. Data should be the same at all centres. Data quality and consistency, as well as ease of use (different data formats, web-interface, quick-look capability, etc.) should be improved.
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A strategy to correct existing records for known breaks and changes should be developed and carried through.
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Current stations have a high density at northern mid-latitudes and in polar regions. There are very few stations in the tropics, or in the Southern Hemisphere.
Variable: Aerosols
Main climate application
Atmospheric aerosols are minor constituents of the atmosphere by mass, but a critical component in terms of impacts on the climate and especially climate changes. Aerosols influence the global radiation balance by directly scattering solar radiation and indirectly through influencing cloud reflectivity, cloud cover and cloud lifetime.
Tropospheric aerosols either originate directly from the surface (sea salt from the oceans, or dust smoke and soot from the continents) or are formed in the atmosphere as a result of complex (photo)chemical processes and reactions between gaseous constituents that themselves originated from the surface (DMS over the oceans, sulphur and nitrogen oxides over the continents). Anthropogenic aerosol influences are considered to have a negative radiative forcing, which on a regional basis may be equal to or greater than the warming associated with greenhouse gases. The IPCC identified anthropogenic aerosols as the most uncertain climate forcing constituent.
The source of most stratospheric aerosols is volcanic eruptions that are strong enough to inject SO2 into the stratosphere. Sources of non-volcanic stratospheric aerosols include carbonyl sulphide (OCS) from oceans, low level SO2 emissions from volcanoes of the Kilauea-type, and various anthropogenic sources, including industrial and perhaps aircraft operations. Measurements of surface and upper-air temperature following the June 1991 eruption of Mt. Pinatubo showed a cooling in globally averaged temperatures at the surface and warming in the stratosphere that lasted for about 2 years. Stratospheric aerosols also provide surfaces on which chemical reactions can occur. The loss of ozone in the lower stratosphere due to heterogeneous chemistry on aerosols or polar stratospheric clouds (PSCs) will cool the Earth’s surface and, therefore, is a negative forcer. The change in cirrus cloud amounts, particle size, and/or lifetime, also have important radiative effects on climate.
Contributing baseline GCOS observations
Aerosol measurements are component for Global Atmospheric Watch (GAW) baseline stations and contribute to the Integrated Global Atmospheric Chemistry Observation (IGACO) theme (whose main purpose is to promote closer co-operation between the space and ground-based measuring communities for atmospheric chemistry). The objective of the GAW aerosol programme is “to determine the spatio temporal distribution of aerosol properties related to climate forcing and air quality up to multi-decadal time scales”. The measurement sites are required to represent the major geographical regions, and to address mainly global climate issues. These regimes include clean and polluted continental, polar, marine, dust impacted, biomass burning and free tropospheric locations. However, chemical composition data or data on precursor species are not readily available for most of these sites and in many cases are not monitored at these locations.
Other contributing observations
Limited networks of sun photometers (e.g. AERONET) have collected relevant observations from which aerosol amounts and properties can be derived. Astronomical observations at night constitute the only long-term recorded archive of atmospheric turbidity, although the latter cannot be directly converted into precise characterizations of aerosol properties and density distributions.
Limited aerosol chemical composition data are available from regional monitoring networks established to deal with acidification issues and from sites operated as part of research programmes. Some regional monitoring sites are GAW regional sites. Regional monitoring networks are largely in mature industrial regions, in North America (e.g. CAPMON, IMPROVE) and in Europe (EMEP). The range of data available from these networks is also limited, e.g., historically only total sulphate levels were determined at EMEP sites. The various continental programmes such as the co-operative programme for monitoring and evaluation of the long-range transmission of air pollutants in Europe (EMEP) and the North American Research Strategy for Tropospheric Ozone (NARSTO) have great potential for complementary contributions to GCOS.
Research orientated sites largely operate as single sites. In the absence of regular inter-comparisons of sampling and analysis methods, which is typically the case, integration of data from these sites is problematic. Research networks such as; AEROCE and ACE-2 Longterm in the North Atlantic, operated by the University of Miami (UM) and the Environment Institute (EI), Joint Research Centre (JRC), Ispra, Italy, respectively and the UM DOE network in the Pacific Ocean, are valuable and unique sources for aerosol chemical composition data for these regions. However, these sites have largely been closed down during the late 1990s.
There are approximately 5 lidar sites in the Northern Hemisphere, that have been making routine laser backscatter measurements of stratospheric aerosols, two stations’ measurements date back to the early 1970s. Also, there are a few sites in the Southern Hemisphere. None, however, are in the tropics. These data are available from (see the Lidar Users Directory) http://iclas.hamptonu.edu. In addition, the University of Wyoming has made routine balloon-borne in situ measurements of stratospheric aerosols in a few size ranges since the early 1970s.
There has been a series of satellite experiments that have made and are still making measurements of stratospheric aerosols on a global basis. The series started with the Stratospheric Aerosol Measurement (SAM)-II instrument launched in 1978, followed by the Stratospheric Aerosol and Gas Experiment (SAGE)-I in 1979, II in 1984 (still operating), and III in 2001. The technique used by all these experiments for aerosol measurements is solar occultation. The data for these experiments reside at the NASA Atmospheric Science Data Center at NASA Langley Research Center, and are available to the community. Significant campaigns and world-wide measurements have been used to validate these data. The world-wide validation data are available at the Langley archive or from the individual investigators.
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